i recommend:
- alien vs. predator 2 (i've never played part one, though)
- system shock 1
and if not for the scaryness then for mere dark atmosphere
- ultima underworld 1 & 2
- halflife 1
- return to castle wolfenstein
EDIT: supporting rhavell's suggestion of clive barker's undying, i encourage
you to try this one first! it's REALLY scary!!
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